The Pharmaceutical and Cosmetic Industries

 

A. Goossens and L. Geusens

 

 

 

Depending on the type of product and exposition, several occupation-induced dermatoses may occur among workers in the pharmaceutical industry.  They include irritation, contact allergy, photo-sensitivity, urticaria, acne venenata, and, less frequently, fixed drug eruption and steroid rosacea (H. Degreef, personal communication), and even toxic epidermal necrolysis (as was the case with the transcutaneous absorption of an intermediary product in the synthesis of tetramisole, an anthelminthic drug.  The dermatoses can be located at the site of contact, which is generally the hand in an occupational context.  Airborne reactions on exposed and non-exposed areas (e.g. by particles trapped under clothing) are not uncommon, and generalized reactions may occur due to inhalation or transcutaneous absorption.  Workers in the pharmaceutical industry are considered to be particularly at risk for irritation and allergic contact dermatitis.  Irritant reactions are frequent but are rarely reported in the literature: occasionally, "epidemics" of such reactions have been described, as was the case in Israel, where pharmaceutical industry workers suffered from burning, erythematous, and vesicular lesions shortly after putting on sterile working clothes.  This was caused by a high residual content (500 ppm!) of ethylene oxide, the recommended safety level being 200 ppm.  An example of occupation-induced non-immunological contact urticaria reactions due to sodium benzoate, notwithstanding the use of protective clothing, gloves, and mask, has been reported.  With regard to contact allergenicity, many substances used in the pharmaceutical industry are very reactive chemically so they are liable to induce not only irritation but also contact sensitization.  The allergenic potential as well as the concentration of the contacted substances are, of course, very important contributing factors.  With a highly allergenic compound, one accidental exposure may cause a chemical burn, primary sensitization, and allergic contact dermatitis.  An example from the pharmaceutical industry was reported: a chemical student working with the synthesis of procaine, accidentally spilled some droplets of p-nitrobenzoyl chloride, a chemical intermediate onto her forearm.  After rinsing with water, an erythematous lesion developed (first-degree burn) that faded the next day.  Two weeks later, however, she presented a non-vesicular erythematous and edematous dermatitis on the same forearm and also the hand.  Patch testing revealed contact allergy to this substance.  In the pharmaceutical industry, people come in contact with both chemical intermediates and finished products.  The risk of developing contact allergy is greatest for chemists and laboratory technicians who are involved in research for new compounds and for cleaning personnel and technicians in general, who are often less well protected than are the workers in production units.  Pharmacists are also exposed to medications when preparing compounded formulations, and the conditions they work in are similar to those of medical personnel.  Here, we will concentrate on the pharmaceutical components responsible for occupation-related contact allergic reactions.  Because little attention has been given in the literature to cosmetic ingredients, we will mention them briefly first.  The test concentrations and vehicles for the allergenic substances and chemical intermediates (listed alphabetically along with their CAS numbers, whenever possible) as reported in the literature are given in Table 1.  The pharmaceutical products described are classified as is in Martindale (1993).

 


Allergens in the cosmetic industry

Methyl heptine carbonate (MHC) and methyl octine carbonate (MOC)

2-bromonitropropanediol

Ylang-ylang oil

Allergens in the pharmaceutical industry

1.       Analgesic and anti-inflammatory agents:        Pyrazinobutazone

2.       Anthelmintics:      Albendazole

Morantel

Piperazine

3.       Anti-arrhythmic agents:         Quinidine sulfate

2,6-dichloropyrimidine

 

4.       Anti-bacterial agents:

 

Penicillins:        Natural penicillins:

Penicillin G or benzylpenicillin

Penicillin V or phenoxymethylpenicillin

 

Semi-synthetic penicillins:         Pivampicillin

Pivmecillinam

Ampicillin

Carbenicillin

Cloxacillin

Mecillinam

 

Cephalosporins:       Cephalothin

Cefamandole

Cefazolin

Cephradine

 

Tetracyclines:          Doxycycline

Methacycline

Oxytetracycline

Tetracycline

 

Macrolides:             Kitasamycin
Midecamycin

 

Aminosides:             Neomycin

Paromomycin

Streptomycin

 

Sulfonamides:          Sulfanilamide

2-aminothiazole

Sulfathiazole


Other antibacterial agents and chemical intermediates from their synthesis:

 

Chloramphenicol and its chemical synthesis intermediates: p-nitrobromacetophenone, p-nitroaminoacetophenone, p-nitroacetamidoacetophenone and p-nitroacetamido-hydroxy propiophenone.

 

Virginiamycin

Colistin

Hydrazine

 

5.       Anti-gout agents:      Ethyl ethoxymethylene cyanoacetate

 

6.       Anti-malarials:       Chloroquine

4,7-dichloroquinoline

Quinine

 

7.       Anti-muscarinic agents:     Biperiden

 

8.             Anti-neoplastic agents and immunosuppressants:

 

Azathioprine

5-chloro-1-methyl-4-nitroimidazole

2,4-diamino-6-chloromethylpteridine hydrochloride (DHC), an intermediary substance in the synthesis of methotrexate.

4-nitrophenyl-N-(2-chloroethyl)carbamate

4-nitrophenyl-N-(2-chloroethyl)-N-nitrosocarbamate

Both of these substances are intermediates in the synthesis of tauromustine.

Cytarabine intermediate

4-amino-5-nitro-6-chloropyrimidine, intermediary product in the synthesis of mercapto-purine.

 

9.       Anti-thyroid agents:    Carbimazole

 

10.         Anti-viral agents:

 

3,4,6- trichloropyridazine

Ethyl-5-acetoxy-6-bromo-2-(bromomethyl)-1-methyl indole-3-carboxylate (SI-4),

an intermediary product in the synthesis of Arbidol, an antiviral medication

11.     Anxiolytic sedatives, hypnotics, and neuroleptics:

 

Chlorpromazine
Perphenazine
P-chlorbenzene sulfonyl glycolic acid nitrile an intermediate from the synthesis of benzodiazepines.
Quinazoline oxide used in the synthesis of chlordiazepoxide.


12.     Beta-adrenoceptor blocking agents:

 

Alprenolol
Metoprolol
Oxprenolol
Propranolol
Epichlorohydrin (a substrate in the synthesis of beta-adrenoceptor blocking agents)
4-amino-alpha-bromo-3,5-dichloroacetophenone by an intermediary product from the synthesis of clenbuterol.

 

13.     Cough suppressants:       Oxolamine

 

14.     Dermatological agents:   Diphencyprone (DPCP)

Squaric acic dibutyl-ester (DBSA)

Coal tar

 

15.     Diuretics:      Bumetanide pro-drugs:     Cl-5-Cl-sulfonyl benzoic acid

4-Cl-5-CL-sulfonyl-3-nitrobenzoic acid

4-Cl-3-nitro-5-sulfonyl benzoic acid

 

16.     Gastro-intestinal agents:

 

Ranitidine

5-[(2-aminoethyl)thiomethyl]-N,N-dimethyl-2-furanmethanamine

1-methylamine-1-methylthio-2-nitroethylene (intermediary substances in the synthesis)

2[4(5)methyl-5(4)-imidazolyl-methyl-thio]-C13 intermediate in the synthesis of H2-antagonists.

 

Chloromethyl heterocyclic intermediates of a histamine antagonist.

4-chloromethyl-2-guanidinothiazole-nitrochloride (FIP)

2-diamino-ethylene-aminothiazolyl-methylenethiourea-dichloride (uranium),

two intermediates from the synthesis of famotidine, an H2-antagonist

Omeprazole

17.     Local anaesthetics:       p-nitrobenzoyl chloride

Procaine

18.     Opoid analgesics:          Morphine

Codeine

Thebaine

19.     Vasodilators:     Nitroglycerin

Trans-methyl-3-(4-methoxyphenyl)glycidate

Methyl 2,3-epoxy-3-(4-methoxyphenyl)propionate chemical intermediates in the synthesis of diltiazem.

Chromonar (or carbocromen)

 


20.         Vitamins:           Retinyl (vitamin A) acetate

Thiamine (vitamin B1)

 

2-methyl-3-nitro-4-methoxymethyl-5-cyano-6-chloropyridine in the synthesis of vitamin.

 

Pyritinol

Cyanocobalamin (vitamin B12)

Vitamin K3  (sodium bisulfite)

Vitamin K4

 

21.         Supplementary drugs and other substances:

 

Nicergoline

10-alpha-methoxy-dihydrolysergo

1-N-methyl-10-alpha-methoxy-dihydrolysergol

Lysergol

Vincamine tartrate

 

22.     Chemical intermediates of various drugs

 

Halogenated molecules:

Chloromethyl imidazoline: an intermediary compound from the synthesis of drugs such as phentolamine (an antihypertensive agent), naphazoline (a sympathomimetic), and antazoline (a histamine-H1-receptor antagonist).

 

Tosyl chloride (p-toluenesulfonyl chloride): an intermediate in the synthesis of pharmaceutical, plastic, and chemical products.  Its hydrolysis into p-toluene sulfonic acid makes it an irritant.

 

4-bromomethyl-6,8-dimethyl-2(1H)-quinolone

4-bromoacetoacet-2,4-dimethylanilide intermediary chemicals in the synthesis of halogenated quinolones and quinolines.

 

2,6-dichloropurine standard intermediary product, widely used in pharmaceutical and other industries.

 

4-chloro-7-nitrobenzofurazan (NBD-CL). This is a reagent used in analytical chemistry.

Diethyl-beta-chloroethylamine (DBCEA).

The two cases of allergic contact dermatitis to this substance described were due to inadequate protective measures and thus accidental contact with these highly irritant and sensitizing pharmaceutical intermediates (Deschamps et al. 1988).

 

Ethyl-2-bromo-p-methoxyfenyl acetate.  This is a derivative of ethyl-p-methoxyfenyl acetate, a frequently used chemical intermediate.

 


Non-halogenated molecules:

Ethylenediamine

2,2 dimethyl-1,3-propane diamine

Intermediary substance C

Butyl acetate

2-aminothiophenol

3,4-dicarboxy hexane-2,5-dione intermediate from the synthesis of a contrast medium used in X-rays produced.

 

N-hydroxyphtalimide (N-HPI)

Dicyclohexyl carbodiimide (DCC)

Diisopropyl carbodiimide (DIC)

Coupling reagents in the pharmaceutical industry, mainly in peptide chemistry, and DCC is also an intermediate in the synthesis of angiotensine.

 

 

Conclusion

 

Occupation-related allergic contact dermatitis is not infrequently observed in the pharmaceutical industry.  If several cases occur in the same company, then the working conditions must be changed to prevent their recurrence.  Measures to be taken include dust control and the installation of closed filter equipment and keeping the workers informed about the potential cutaneous and other risks associated with the manipulation of the chemicals they are likely to come in contact with.  Moreover, individual protective measurements - adequate protecting gloves, clothing, mask, and, if necessary boots - followed by close monitoring of their effectiveness, are also necessary.

 

Appendix: Summary Table

Allergen patch test concentration vehicle

Albendazole (54965-21-8) 3.8 % and 1.9 %; 1 % Suspension Petrolatum

10-alfa-methoxy-dihydrolysergol 7 % Ethanol

Alprenolol (13655-52-2) 1 %; 0.5 %; 0.25 % and 0.125 % Water

4-amino-alfa-bromo-3,5-dichloroacetophenone 1 % and 0.5 % Petrolatum

5[(2-aminoethyl)thiomethyl]-N,N-dimethyl-2-furanmethanamine 1 % Water

4-amino-5-nitro-6-chloropyrimidine ??

2-aminothiazole (96-50-4) ??

2-aminothiophenol (137-07-5) 0.1 %; 0.01 % and 0.001 % Petrolatum

Ampicillin (69-53-4) 20 %; 5 %; 1 % and 0.1 % Petrolatum

Azathioprine (446-86-6) 1 % and 0.1 % Petrolatum

Biperiden (514-65-8) 1 % Petrolatum

4-bromoacetoacet-2,4-dimethylanilide 1 % and 0.1 % Petrolatum

4-bromomethyl-6,8-dimethyl-2(1H)-quinolone 1 % and 0.1 % Petrolatum

2-bromo-2-nitro-1,3-propanediol (52-51-7) 0.5 % Petrolatum


Butyl acetate (123-86-4) 5 % Olive oil

Carbenicillin (4800-94-6) 20 % Petrolatum

Carbimazole (22232-54-8) 50 %; 25 % and 10 % Pet. + UVA

Cephalotin (58-71-9) 5 % and 1 % Water

Allergen patch test concentration vehicle

Cefamandole (30034-03-8) 5 % Water

Cefazolin (27164-46-1) 5 % and 1 % Water

Cephradine (38821-53-3) 20 % Petrolatum

Chloramphenicol (56-75-7) 5 % and 1 % Petrolatum

p-chlorbenzene sulfonyl glycolic acid nitrile ??

Chloromethyl imidazoline 0.001 % and 0.0001 % Water

Chlorpromazine (50-53-3) 1 %; 0.001 % Pet. + UVA

4-chloro-5-chloro-sulfonyl benzoic acid 1 % Petrolatum

4-chloro-5-chloro-sulfonyl-3-nitrobenzoic acid 1 % Petrolatum

4-chloromethyl-2-guanidothiazole-nitrochloride1 % Water

Chloromethyl heterocyclic intermediates 1 % and 0.1 % Petrolatum

5-chloro-1-methyl-4-nitroimidazole 10 %; 1 %; 0.1 % and 0.01 % Petrolatum

4-chloro-7-nitro-benzofurazan 0.1 %; 0.05 % and 0.01 % Petrolatum

4-chloro-3-nitro-5-sulfonyl benzoic acid 1 % Petrolatum

Chloroquine (54-05-7) 1 % Petrolatum

Chromonar (804-10-4) 1 % Water

Cloxacillin (7081-44-9) 20 % and 1 % Petrolatum

Codeinephosphate hydrochloride (76-57-3) 1 %; 1 % Water Petrolatum

 

Allergen patch test concentration vehicle

 

Colistin (1066-17-7) 1.000.000 U/g

Cyanocobolamin (68-19-9) 10 % Petrolatum

Cytarabine intermediate 1 %; 0.5 % and 0.1 % Water

2,4-diamino-6-chloromethylpteridine HCL 1 %; 0.1 % and 0.01 % Petrolatum

2-diamino-ethylene-aminothiazolyl-methylene-nitrourea-dichloride 1 % Water

3,4-dicarboxyhexane-2,5-dione 1 %; 0.1 %, 0.032 %; 0.01 % and 0.0032 % Acetone

2,6-dichloropurine (5451-40-1) 1 % Petrolatum

2,6-dichloropyrimidine (3934-20-1) ??

4,7-dichloroquinoline (86-98-6) 5 % Petrolatum

Dicyclohexyl carbodiimide (538-75-0) 0.1 % Acetone or Petrolatum

Diethyl-beta-chloroethylamine as is

Diisopropyl carbodiimide (693-13-0) 0.2 % Acetone

2,2-dimethyl-1,3-propane diamine 2 % Petrolatum

Diphencyprone (886-38-4) 0.01 % Acetone

Doxycycline (10592-13-9) 10 % Petrolatum

Epichlorohydrin (106-89-8) 0.001 % Water

Ethyl-5-acetoxy-6-bromo-2-(bromomethyl)-1-methyl indole-3-carboxylaat 0.1 % Petrolatum

 


Allergen patch test concentration vehicle

 

Ethyl-2-bromo-p-methoxyphenyl acetate 10 %; 1 %; 0.1 % and 0.01 % Ethanol

Ethylenediamine (107-15-3) 1 % Petrolatum

Ethylethoxymethylene cyanoacetate 0.01 % Petrolatum

Hydrazine (302-01-2) 1 % Petrolatum

N-hydroxyphtalimide (524-38-9) 0.001 % Ethanol

Kitasamycin Kitasamycintartrate as is 4 % Water

Coal tar 5 % Petrolatum

Lysergol 7 % Ethanol

Mecillinam 10 % and 1 % Petrolatum

Menadiol (481-85-6) 0.1 % Olive oil

Menadione (58-27-5)

Menadione sodium bisulfite (57414-02-5) 0.1 % 0.1 % Olive oil Petrolatum

Methacycline (3963-95-9) 10 % Petrolatum

1N-methyl-10-alfa-methoxy dihydrolysergol 7 % Ethanol

1-methylamine-1-methylthio-2-nitroethylene 1 % and 0.5 % Petrolatum

Methyl 2,3-epoxy-3-(4-methoxyphenyl)propionate 1 % Ethanol

Methyl heptinecarbonate 1 % MEK

2[4(5)methyl-5(4)-imidazolyl-methyl-thio]-C 131 % and 0.1 % Water or Ethanol

Allergen patch test concentration vehicle

 

2-methyl-3-nitro-4-methoxymethyl-5-cyano-6-chloro-pyridine ??

Methyl octinecarbonate1 % MEK

Midecamycin (35457-80-8) as such

Morantel (20574-50-9) 5 % and 1 % Petrolatum

Morphine (57-27-2) 1 % 10 % and 5 % Ethanol Water

Neomycin sulfate (1404-04-2) 20 % Petrolatum

Nicergoline (27848-84-6) 7 % Ethanol

p-nitroacetamidoacetophenone 1 % Ethanol

p-nitroacetamido-hydroxypropiophenone 0.5 % Ethanol

p-nitroamino-acetophenone 1 % Methylalcohol

p-nitrobenzoyl chloride (122-04-3) 3 % and 1 % Petrolatum

p-nitrobromacetophenone 0.1 % Ethanol

Nitroglycerin (55-63-0) 0.02 % 2 % Water Petrolatum

4-nitrophenyl-N-(2-chloroethyl)carbamate 0.01 %; 0.001 % and 0.0001 % Water

4-nitrophenyl-N-(2-chloroethyl)-N-nitrosocarbamate 0.01 % and 0.001 % Water

Omeprazole (73590-58-6) 1 %; 0.5 % and 0.25 % 1 %; 0.5 % and 0.1 % Petrolatum Ethanol

Allergen patch test concentration vehicle

 

Oxolamine (959-14-8) 0.5 % and 0.1 % Water (+ Ethanol)

Oxprenolol (6452-71-7) 1 % Petrolatum

Oxytetracycline (6153-64-6) 10 % Petrolatum

Paromomycin (1263-89-4) 20 % Petrolatum

Penicillin G (1538-09-6) 3.000.000 U/g 10 % and 1 % Petrolatum

Penicillin V (87-08-1) 10 % and 1 % Petrolatum

Perphenazine (58-39-9) 0.01 % Pet. + UVA


Piperazine (110-85-0) 1 %; 0.5 % and 0.1 % Petrolatum

Pivampicillin base (33817-20-8) 5 % Petrolatum

Pivmecillinam 10 % Petrolatum

Procaine (59-46-1) 2 % Water

Promethazine (58-33-3) 1 % Petrolatum

Propranolol (525-66-6) 1 % Petrolatum

Pyrazinobutazone 5 % and 1 % Petrolatum

Pyritinol (1098-97-1) 2 % Water

Quinazoline oxide (253-82-7) 1 % Petrolatum

Quinidine sulfate (50-54-4) 0.5 % Water

Allergen patch test concentration vehicle

 

Quinine alkaloid (130-95-0) dihydrochloride 1 % Petrolatum Water

Ranitidine (66357-35-5) 10 %; 5 %; 2 %; 1 % and 0.1 % Petrolatum

Retinyl acetate (127-47-9) 0.5 % and 0.1 % Petrolatum

Squaric acid dibutyl-ester 0.02 % Petrolatum

Streptomycin (57-92-1) 10 % and 1 % Water

Sulfanilamide (63-74-1) 5 % Petrolatum

Tetracycline (60-54-8) 10 % Petrolatum

Thebaine (115-37-7) 5 % Ethanol

Thiamine (59-43-8) 10 % and 5 % Water

Thiothiamine 5 % and 1 % Water

Tosyl-chloride (98-59-9) 1 % Ethanol

Trans-methyl-3-(4-methoxyphenyl)glycidate 10 %; 1 % and 0.5 % Petrolatum

3,4,6-trichloropyridazine 1 % Petrolatum

Vincamine tartrate (1617-90-9) 1 % Water

Virginiamycin (M1: 21411-53-0) (S1: 23152-29-6) 5 % Petrolatum

Ylang-ylang oil 2 % Petrolatum

 

 

Reference

 

Goossens A, Geusens L.  The Pharmaceutical and Cosmetic Industries.  Chapter 163.  In: Handbook of Occupational Dermatology.  Kanerva L, Elsner P, Wahlberg JE, Maibach HI (eds.), Springer-Verlag, Berlin, Heidelberg 2000, pp 1041-1052.

 

 

Key words:     cosmetic - occupational - pharmaceutical